Influence of flue gas on the catalytic activity of an immobilized aluminium (salen) complex for cyclic carbonate synthesis

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  2. Professor Michael North
  3. Dr Carl Young
Author(s)North M, Wang B, Young C
Publication type Article
JournalEnergy & Environmental Science
Year2011
Volume4
Issue10
Pages4163-4170
ISSN (print)1754-5692
ISSN (electronic)1754-5706
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The impact of flue gas from the combustion of natural gas or coal in a combustion test facility on the activity of catalysts for the synthesis of cyclic carbonates from epoxides and waste carbon dioxide has been investigated. In batch reactions with styrene oxide as substrate, some loss of catalyst activity was apparent and this was greater for catalyst exposed to flue gas generated from burning coal than for catalyst exposed to flue gas obtained by burning gas. In a gas-phase flow reactor with ethylene oxide as substrate, the detrimental effect of flue gas exposure on catalyst activity was much less apparent.
PublisherRoyal Society of Chemistry
URLhttp://dx.doi.org/10.1039/c1ee01074c
DOI10.1039/c1ee01074c
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